Login | Register

Harmonic states in quantum cascade lasers: Frequency-domain analysis and mode-spacing control

Title:

Harmonic states in quantum cascade lasers: Frequency-domain analysis and mode-spacing control

Roy, Mithun (2021) Harmonic states in quantum cascade lasers: Frequency-domain analysis and mode-spacing control. Masters thesis, Concordia University.

[thumbnail of Roy_MASc_F2021.pdf]
Preview
Text (application/pdf)
Roy_MASc_F2021.pdf - Accepted Version
Available under License Spectrum Terms of Access.
3MB

Abstract

Quantum cascade lasers (QCLs) are unipolar lasers where lasing transition and carrier transport occur between subbands that result from multiple nanometer-thick quantum wells and barriers formed by the conduction band edges of a semiconductor heterostructure. Since their inception in 1994, QCLs have undergone tremendous improvements with respect to output power, frequency range covered, and maximum operating temperature. As a result, they have become a prominent source of light emitting in the mid- and far-infrared regions of the electromagnetic spectrum.

Multimode behavior of QCLs was a focus of many past works. In a recent comprehensive study, it was found that, if the pumping is increased gradually from threshold, QCLs enter into a harmonic state regime, which is characterized by the lasing of side modes that are separated from each other by multiples of free spectral range (FSR). With a further increase in the pumping, finally, transition into the familiar single-FSR-spaced regime (dense state regime) occurs. Unlike the dense state regime, the harmonic state regime of QCLs has not gone through intense scrutiny, as it is a relatively recent discovery.

In this thesis, a theoretical investigation into the harmonic state regime of QCLs is performed. The work is based on Maxwell’s equation and the density matrix (DM) formalism. The two-level DM equations, although commonly employed, ignore many important details of complex carrier transport through a QCL structure. Therefore, here, a three-level DM formalism is employed, which takes into account phenomena such as resonant tunneling and carrier scattering between the three states.

The thesis is mainly divided into two parts. In the first part, starting from the DM-Maxwell equations, an analytical expression for the instability gain of the side modes is derived. This expression can explain the appearance of harmonic states in QCLs. Using this analytical expression, the effects of group velocity dispersion on the harmonic states are studied. In the second part, multimode behavior of QCLs is analyzed using a more general model than that used in the first part. In particular, openness (non-unity facet reflectivity) of the cavity is considered, which was not taken into account in previous works that used the modal expansion method to study QCLs. Using the theory, it is shown that the coating of a facet can be used to excite harmonic states with different mode spacing. Such a control over the generation of harmonic states could make QCLs invaluable for applications such as microwave and terahertz generation, picosecond pulse generation in the mid-infrared frequency range, and broadband spectroscopy.

Divisions:Concordia University > Gina Cody School of Engineering and Computer Science > Electrical and Computer Engineering
Item Type:Thesis (Masters)
Authors:Roy, Mithun
Institution:Concordia University
Degree Name:M.A. Sc.
Program:Electrical and Computer Engineering
Date:2 August 2021
Thesis Supervisor(s):Kabir, M. Z.
Keywords:Quantum cascade lasers, harmonic states, four-wave mixing, open cavity, constant-flux states, facet engineering
ID Code:988722
Deposited By: Mithun Roy
Deposited On:30 Nov 2021 20:53
Last Modified:20 Aug 2023 00:00

References:

[1] A. E. Siegman, Lasers (University Science Books, 1986).

[2] D. J. Griffiths, Introduction to Quantum Mechanics (Prentice Hall, 1995).

[3] P. Tzenov, “Modeling and simulations of quantum cascade lasers for frequency comb generation,” Ph.D. dissertation (Technical University of Munich, 2019).

[4] B. Williams, “Terahertz quantum-cascade lasers,” Nat. Photonics 1, 517–525 (2007).

[5] R. F. Kazarinov and R. A. Suris, “Possibility of the amplification of electromagnetic waves in a semiconductor with a superlattice,” Soviet Physics-Semiconductors 5, 707–709 (1971).

[6] J. Faist, F. Capasso, D. L. Sivco, C. Sirtori, A. L. Hutchinson, and A. Y. Cho, “Quantum cascade laser,” Science 264, 553–556 (1994).

[7] M. Beck, D. Hofstetter, T. Aellen, J. Faist, U. Oesterle, M. Ilegems, E. Gini, and H. Melchior, “Continuous wave operation of a mid-infrared semiconductor laser at room temperature,” Science 295, 301–305 (2002).

[8] R. Kohler, A. Tredicucci, F. Beltram, H. Beere, E. Linfield, A. Davies, D. Ritchie, R. Iotti, and F. Rossi, “Terahertz semiconductor-heterostructure laser,” Nature 417, 156–159 (2002).

[9] A. Khalatpour, A. K. Paulsen, C. Deimert, Z. R. Wasilewski, and Q. Hu, “High-power portable terahertz laser systems,” Nat. Photonics 15, 16–20 (2021).

[10] A. Bismuto, R. Terazzi, M. Beck, and J. Faist, “Electrically tunable, high performance quantum cascade laser,” Appl. Phys. Lett. 96, 141105 (2010).

[11] F. Xie, C. G. Caneau, H. P. LeBlanc, M. T. Ho, J. Wang, S. Chaparala, L. C. Hughes, and C. -e. Zah, “High power and high temperature continuous-wave operation of distributed Bragg reflector quantum cascade lasers,” Appl. Phys. Lett. 104, 071109 (2014).

[12] D. Kazakov, M. Piccardo, Y. Wang, P. Chevalier, T. S. Mansuripur, F. Xie, C.-e. Zah, K. Lascola, A. Belyanin, and F. Capasso, “Self-starting harmonic frequency comb generation in a quantum cascade laser,” Nat. Photonics 11, 789–792 (2017).

[13] T. S. Mansuripur, C. Vernet, P. Chevalier, G. Aoust, B. Schwarz, F. Xie, C. Caneau, K. Lascola, C. Zah, D. P. Caffey, T. Day, L. J. Missaggia, M. K. Connors, C. A. Wang, A. Belyanin, and F. Capasso, “Single-mode instability in standing-wave lasers: The quantum cascade laser as a self-pumped parametric oscillator,” Phys. Rev. A 94, 063807 (2016).

[14] M. Piccardo, P. Chevalier, T. S. Mansuripur, D. Kazakov, Y. Wang, N. A. Rubin, L. Meadowcroft, A. Belyanin, and F. Capasso, “The harmonic state of quantum cascade lasers: origin, control, and prospective applications [Invited],” Opt. Express 26, 9464–9483 (2018).

[15] A. Hugi, G. Villares, S. Blaser, H. Liu, and J. Faist, “Mid-infrared frequency comb based on a quantum cascade laser,” Nature 492, 229–233 (2012).

[16] D. Burghoff, T.-Y. Kao, N. Han, C.W. I. Chan, X. Cai, Y. Yang, D. J. Hayton, J.-R. Gao, J. L. Reno, and Q. Hu, “Terahertz laser frequency combs,” Nat. Photonics 8, 462–467 (2014).

[17] M. Piccardo, B. Schwarz, D. Kazakov, M. Beiser, N. Opacak, Y. Wang, S. Jha, J. Hillbrand, M. Tamagnone, W. T. Chen, A. Y. Zhu, L. L. Columbo, A. Belyanin, and F. Capasso, “Frequency combs induced by phase turbulence,” Nature 582, 360–364 (2020).

[18] J. H. Davies, The Physics of Low-Dimensional Semiconductors (Cambridge University Press, 1998).

[19] J. Faist, F. Capasso, C. Sirtori, D. L. Sivco, J. N. Baillargeon, A. L. Hutchinson, S.‐N. G. Chu, and A. Y. Cho, “High power mid‐infrared ( ) quantum cascade lasers operating above room temperature,” Appl. Phys. Lett. 68, 3680–3682 (1996).

[20] J. Faist, Quantum Cascade Lasers (Oxford University Press, 2013).

[21] R. W. Boyd, Nonlinear Optics, 3rd ed. (Academic, 2008).

[22] M. A. Talukder, “Modeling of gain recovery of quantum cascade lasers,” J. Appl. Phys. 109, 033104 (2011).

[23] M. Roy and M. Z. Kabir, “Harmonic instability in a quantum cascade laser with Fabry-Perot cavity,” J. Appl. Phys. 128, 043105 (2020).

[24] H. Risken and K. Nummedal, “Self‐Pulsing in Lasers,” J. Appl. Phys. 39, 4662–4672 (1968).

[25] R. Graham and H. Haken, “Quantum theory of light propagation in a fluctuating laser-active medium,” Z. Phys. A: Hadrons Nucl. 213, 420–450 (1968).

[26] C. Y. Wang, L. Diehl, A. Gordon, C. Jirauschek, F. X. Kartner, A. Belyanin, D. Bour, S. Corzine, G. Hofler, M. Troccoli, J. Faist, and F. Capasso, “Coherent instabilities in a semiconductor laser with fast gain recovery,” Phys. Rev. A 75, 031802 (2007).

[27] A. Gordon, C. Y. Wang, L. Diehl, F. X. Kartner, A. Belyanin, D. Bour, S. Corzine, G. Hofler, H. C. Liu, H. Schneider, T. Maier, M. Troccoli, J. Faist, and F. Capasso, “Multimode regimes in quantum cascade lasers: from coherent instabilities to spatial hole burning,” Phys. Rev. A 77, 053804 (2008).

[28] N. Vukovic, J. Radovanovic, V. Milanovic, and D. L. Boiko, “Analytical expression for Risken-Nummedal Graham-Haken instability threshold in quantum cascade lasers,” Opt. Express 24, 26911–26929 (2016).

[29] N. N. Vukovic, J. Radovanovic, V. Milanovic, and D. L. Boiko, “Low-Threshold RNGH Instabilities in Quantum Cascade Lasers,” IEEE J. Sel. Top. Quantum Electron. 23, 1200616 (2017).

[30] H. Li, P. Laffaille, D. Gacemi, M. Apfel, C. Sirtori, J. Leonardon, G. Santarelli, M. Rosch, G. Scalari, M. Beck, J. Faist, W. Hansel, R. Holzwarth, and S. Barbieri, “Dynamics of ultra-broadband terahertz quantum cascade lasers for comb operation,” Opt. Express 23, 33270 (2015).

[31] G. Villares and J. Faist, “Quantum cascade laser combs: effects of modulation and dispersion,” Opt. Express 23, 1651–1669 (2015).

[32] S. T. Hendow and M. Sargent III, “Theory of single-mode laser instabilities,” J. Opt. Soc. Am. B 2, 84–101 (1985).

[33] R. Terazzi, T. Gresch, A. Wittmann, and J. Faist, “Sequential resonant tunneling in quantum cascade lasers,” Phys. Rev. B 78, 155328 (2008).

[34] R. Terazzi, T. Gresch, A. Wittmann, and J. Faist, “Erratum: Sequential resonant tunneling in quantum cascade lasers [Phys. Rev. B 78, 155328 (2008)],” Phys. Rev. B 83, 039902 (2011).

[35] M. Sargent III, M. O. Scully, and W. E. Lamb Jr., Laser Physics (Addison-Wesley, 1974).

[36] Y. K. Chembo and N. Yu, “Modal expansion approach to optical-frequency-comb generation with monolithic whispering-gallery-mode resonators,” Phys. Rev. A 82, 033801 (2010).

[37] N. Opacak and B. Schwarz, “Theory of Frequency-Modulated Combs in Lasers with Spatial Hole Burning, Dispersion, and Kerr Nonlinearity,” Phys. Rev. Lett. 123, 243902 (2019).

[38] Y. Wang and A. Belyanin, “Active mode-locking of mid-infrared quantum cascade lasers with short gain recovery time,” Opt. Express 23, 4173–4185 (2015).

[39] C. Jirauschek and T. Kubis, “Modeling techniques for quantum cascade lasers,” Appl. Phys. Rev. 1, 011307 (2014).

[40] A. Wittmann, Y. Bonetti, J. Faist, E. Gini, and M. Giovannini, “Intersubband linewidths in quantum cascade laser designs,” Appl. Phys. Lett. 93, 141103 (2008).

[41] Y. Wang and A. Belyanin, “Harmonic frequency combs in quantum cascade lasers: Time-domain and frequency-domain theory,” Phys. Rev. A 102, 013519 (2020).

[42] M. Piccardo, P. Chevalier, S. Anand, Y. Wang, D. Kazakov, E. A. Mejia, F. Xie, K. Lascola, A. Belyanin, and F. Capasso, “Widely tunable harmonic frequency comb in a quantum cascade laser,” Appl. Phys. Lett. 113, 031104 (2018).

[43] F. Wang, V. Pistore, M. Riesch, H. Nong, P.-B. Vigneron, R. Colombelli, O. Parillaud, J. Mangeney, J. Tignon, C. Jirauschek, and S. S. Dhillon, “Ultrafast response of harmonic modelocked THz lasers,” Light: Sci. Appl. 9, 51 (2020).

[44] A. Forrer, Y. Wang, M. Beck, A. Belyanin, J. Faist, and G. Scalari, “Self-starting harmonic comb emission in THz quantum cascade lasers,” Appl. Phys. Lett. 118, 131112 (2021).

[45] P. Tzenov, D. Burghoff, Q. Hu, and C. Jirauschek, “Time domain modeling of terahertz quantum cascade lasers for frequency comb generation,” Opt. Express 24, 23232–23247 (2016).

[46] D. Burghoff, “Unraveling the origin of frequency modulated combs using active cavity mean-field theory,” Optica 7, 1781–1787 (2020).

[47] J. B. Khurgin, Y. Dikmelik, A. Hugi, and J. Faist, “Coherent frequency combs produced by self frequency modulation in quantum cascade lasers,” Appl. Phys. Lett. 104, 081118 (2014).

[48] H. E. Tureci, A. D. Stone, and B. Collier, “Self-consistent multimode lasing theory for complex or random lasing media,” Phys. Rev. A 74, 043822 (2006).

[49] H. E. Tureci, A. D. Stone, and L. Ge, “Theory of the spatial structure of nonlinear lasing modes,” Phys. Rev. A 76, 013813 (2007).

[50] H. E. Tureci, L. Ge, S. Rotter, and A. D. Stone, “Strong interactions in multimode random lasers,” Science 320, 643–646 (2008).

[51] L. Ge, R. J. Tandy, A. D. Stone, and H. E. Tureci, “Quantitative verification of ab initio self-consistent laser theory,” Opt. Express 16, 16895–16902 (2008).

[52] L. Ge, Y. D. Chong, and A. D. Stone, “Steady-state ab initio laser theory: generalizations and analytic results,” Phys. Rev. A 82, 063824 (2010).

[53] O. Zaitsev and L. Deych, “Recent developments in the theory of multimode random lasers,” J. Opt. 12, 024001 (2010).

[54] A. Cerjan, Y. D. Chong, L. Ge, and A. D. Stone, “Steady-state ab initio laser theory for n-level lasers,” Opt. Express 20, 474–488 (2012).

[55] A. Cerjan and A. D. Stone, “Steady-state ab initio theory of lasers with injected signals,” Phys. Rev. A 90, 013840 (2014).

[56] A. Cerjan, Y. D. Chong, and A. D. Stone, “Steady-state ab initio laser theory for complex gain media,” Opt. Express 23, 6455–6477 (2015).

[57] O. Zaitsev and L. Deych, “Diagrammatic semiclassical laser theory,” Phys. Rev. A 81, 023822 (2010).

[58] L. Ge, “Steady-state ab initio laser theory and its applications in random and complex media,” Ph.D. dissertation (Yale University, 2010).
All items in Spectrum are protected by copyright, with all rights reserved. The use of items is governed by Spectrum's terms of access.

Repository Staff Only: item control page

Downloads per month over past year

Research related to the current document (at the CORE website)
- Research related to the current document (at the CORE website)
Back to top Back to top